Have you read The Probabilistic Method by Joel Spencer and Noga Alon?
Although originally developed by Erdos, here's an example of the probabilistic method taken from combinatoricist Po-Shen Loh:
A1,dots,Assubseteq1,2,dots,M such that AinotsubsetAj and let ai=|Ai|. Show that sumsi=1frac1binomMaileq1
The hint is to consider a random permutation sigma=(sigma1,dots,sigmaM). Loh defines the event Ei when sigma1,dots,sigmaai=Ai. Then he observes the events Ei are mutually exclusive and that mathbbP(Ei) is relevant to our problem...
There are probably a lot of olympiad combinatorics problems that can be solved this way. Err... you were asking for number theory, but you will find both in Spencer and Alon's book.
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